Disturbing the Fermi Sea with Rydberg States – Physics

May 17, 2021• Physics 14, 74

A method that enables long-range interactions between fermions on a lattice allows atomic quantum simulations of exotic quantum many-body phenomena.

Currently, one of the best ways to model complex quantum systems is through atomic quantum simulations. Controlling interactions between atoms is key to such simulations, something that can be achieved in atomic lattices using the well-established Feshbach-resonance approach. While that approach can be used to vary the strength of short-range interactions between atoms, it does not carry over to long-range interactions, leaving some interesting quantum systems outside of the techniques scope. Elmer Guardado-Sanchez at Princeton University and colleagues have now shown that such long-range interactions can be controlled using Rydberg dressing in a lattice of lithium ( 6Li) atoms [1]. The teams demonstration opens up unprecedented opportunities for exploring systems that exhibit rich fermionic many-body physics.

In the Feshbach-resonance approach to interaction control, a variable magnetic field is used to tune the scattering dynamics of colliding atoms. The use of this technique has led to the experimental observation of the crossover between the Bose-Einstein-condensation (BEC) regimein which strongly interacting fermions form bosonic moleculesand the Bardeen-Cooper-Schrieffer (BCS) regimein which weakly interacting fermions form loosely bound Cooper pairs. Quantum phenomena that can be simulated using such interactions range from the electron correlations behind high-temperature superconductors to the quantum kinematics taking place in distant neutron stars. Despite this versatility, there remains an important class of systems beyond the reach of simulations based on local interactions. Those systems are ones composed of spinless fermions, which the Pauli exclusion principle forbids from sitting on top of one another, making local interactions largely irrelevant. Instead, it is the long-range interactions that must be controlled.

One way to engineer such long-range interactions between spinless atomic fermions is to excite the atoms to Rydberg states, in which an electron occupies a high orbital. This method has been proposed theoretically as a way to mediate correlated topological density waves within a fermionic system [2]. Guardado-Sanchez and colleagues now employ the technique experimentally, which they do with an ensemble of spinless, fermionic 6Li atoms.

The team cooled a dilute gas of 6Li atoms in an optical lattice to a quantum degenerate temperature, one where each atoms de Broglie wavelength becomes larger than the interatomic spacing. Unable to reach the ground state simultaneously (because of the Pauli exclusion principle), the atoms freeze one by one at the lowest momentum available, forming a Fermi sea (Fig. 1). In this sea state, the atoms barely interact, and there are both minimal thermal and minimal quantum fluctuations.

The teams next step was to use a laser to implement a Rydberg dressing scheme, which mixes the systems internal ground state with a highly excited Rydberg state. An atom in a Rydberg state exhibits a larger electric dipole moment than one in the ground state because of the greater distance between its ion core and its outermost electron. This dipole-moment enhancement produces an effective soft-core interaction between Rydberg-dressed atoms, meaning that the interaction strength remains roughly constant as the interparticle distance increases, before dropping off above a threshold length scale [24]. The researchers show that they can manipulate the strength and the range of this interaction by varying the intensity and frequency of the laser. Although the Rydberg-dressing-induced interaction is isotropic across the two-dimensional system, the motion (by quantum tunneling) of the fermions is restricted to one dimension. This limited freedom of motion hinders the infamous Rydberg-avalanching-loss process by which Rydberg atoms collide, gain kinetic energy, and escape the trap.

The long-range interaction and the consequent hopping motion of the fermions generate many-body excitationscommonly called quantum fluctuationson top of the Fermi sea. These collective quantum fluctuations can have tremendously rich features, yielding many kinds of quantum-correlated states of matter. The types of phenomena that arise in such a system of interacting fermions depend on the way in which the fermions pair up, or, more precisely, on the momenta of the participating fermions and the Cooper pairs that result. These momentum-dependent interactions, in turn, are governed largely by the range of the interaction relative to the lattice spacing. A soft-core interaction with a tunable length, such as that realized by Guardado-Sanchez and colleagues, could lead to abundant momentum-dependent behaviors, generating, for example, topological density waves [2] and chiral p+ip superfluidity [5]. Such p+ip superfluids support topological Majorana vortices and offer a plausible route toward realizing topological quantum computation.

Even more exotic and counterintuitive phenomena may arise when different pairing possibilities occur simultaneously. For example, although mean-field theories typically predict that superfluidity appears in the presence of purely attractive interactions, functional renormalization group calculations suggest that a complex combination of different fermion pairings should generate unconventional f-wave superfluidity even with atomic repulsion [6]. Guardado-Sanchez and colleagues have so far only demonstrated attractive interactions, but tuning from attraction to repulsion is experimentally feasible [7]. Interesting effects should also arise when the interaction strength completely dominates the kinetic energy, with the system then being driven toward a Wigner crystal or fractional quantum Hall state [8, 9].

In the teams experiment, with its lattice-hopping fermions, the dynamical aspects of the system are more easily observed than the quantum many-body equilibrium states. Uncovering how to probe such states in a nonequilibrium setting should stimulate future theoretical investigation. On the application side, as well as the above-mentioned potential for topological quantum computing, long-range interaction control is a key step toward performing quantum simulations of quantum chemistry problems. Such simulations represent one arena ripe for applications employing the so-called quantum advantage to solve problems that would be intractable using classical computers. One strength of the teams scheme in realizing applications is that, unlike previously developed Feshbach-resonance techniques, it is magnetic-field-free. This aspect provides extra freedom to integrate the technique with certain magnetic-field-sensitive cold-atom quantum technologies, such as artificial gauge fields.

Xiaopeng Li is professor of physics in the Physics Department of Fudan University, China, jointly employed by Shanghai Qi Zhi Institute. He is active in quantum information science and condensed-matter theories, with his primary research interests in exploiting the quantum computation power of various quantum simulation platforms. He received his Ph.D. in physics from the University of Pittsburgh in 2013 and joined Fudan University as a faculty member in 2016 after three years at the University of Maryland, supported by a Joint Quantum Institute theoretical postdoctoral fellowship. He has been a full professor since 2019.

Elmer Guardado-Sanchez, Benjamin M. Spar, Peter Schauss, Ron Belyansky, Jeremy T. Young, Przemyslaw Bienias, Alexey V. Gorshkov, Thomas Iadecola, and Waseem S. Bakr

Phys. Rev. X 11, 021036 (2021)

Published May 17, 2021

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Disturbing the Fermi Sea with Rydberg States - Physics